V‐Shaped Methylpyrimidinium Chromophores for Nonlinear Optics

Synthesis of TiO2-ZnO-ZrO2 Nanocomposites for Nonlinear Optics Applications

A sol-gel technique under ultrasonic irradiation was applied to synthesize ZrO2/TiO2/ZnOnanocomposites. X-ray diffraction analysis confirmed the successful synthesis of nanocomposites. The strain and crystalline size values of ZrO2/TiO2/ZnO nanocomposites are estimated to be 9.98×10-4 and 17.66 nm, respectively. The linear absorption coefficient of ZrO2/TiO2/ZnO nanocomposites was measure...

Nonlinear Optics Basics: Kramers-Krönig Relations in Nonlinear Optics

Nonlinear optical chromophores as nanoscale emitters for single-molecule spectroscopy.

Fluorescence imaging of single molecules at room temperature is a powerful technique for studying complex condensed phase systems and revealing structure and dynamics hidden by ensemble measurements. Successful single-molecule spectroscopic experiments rely upon strong emitters that can be detected at the level of individual copies above the relevant background signals. This Account discusses a...

Dispersive nonlinear geometric optics

We construct infinitely accurate approximate solutions to systems of hyperbolic partial differential equations which model short wavelength dispersive nonlinear phenomena. The principal themes are the following. ~1! The natural framework for the study of dispersion is wavelength e solutions of systems of partial differential operators in e]. The natural e-characteristic equation and e-eikonal e...

Twinning and Nonlinear Optics

A comprehensive theory of quasi-phase-matched (QPM) three-wave interactions in twinned plates of q3m semiconductors is developed. The 180* phase change required by QPM is studied by treating the nonlinear polarization as a bilinear form in the applied electric field and decomposing it into invariant and sign changing parts under a 2-fold rotation of an arbitrary crystal lattice. A new 3 X 3 mat...